Uranium capture by a layered 2D/2D niobium phosphate/holey graphene architecture via an electro-adsorption and electrocatalytic reduction coupling process

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成果类型：

期刊论文

作者：

Liao, Yun*;Lei, Ruilin;Weng, Xiaofang;Yan, Chuan;Fu, Jiaxi;...

通讯作者：

Liao, Yun;Wang, Meng;Wang, Hongqing

作者机构：

[Weng, Xiaofang; Fu, Jiaxi; Lei, Ruilin; Zhang, Chen; Wei, Guoxing; Liao, Yun] Univ South China, Sch Chem & Chem Engn, Hengyang 421001, Hunan, Peoples R China.

[Wang, Hongqing; Liao, Yun] Univ South China, Hunan key Lab Design & Applicat Actinide Complexes, Hengyang 421001, Hunan, Peoples R China.

[Yan, Chuan; Wang, Meng] Univ South China, Sch Nucl Sci & Technol, Hengyang 421001, Hunan, Peoples R China.

通讯机构：

[Wang, Hongqing; Liao, Yun] H

[Wang, Meng] S

Hunan key laboratory for the design and application of actinide complexes, University of South China, Hengyang, Hunan 421001, PR China. Electronic address:

School of Nuclear Science and Technology, University of South China, Hengyang, Hunan 421001, China. Electronic address:

Hunan key laboratory for the design and application of actinide complexes, University of South China, Hengyang, Hunan 421001, PR China. Electronic address:

语种：

英文

关键词：

Electro-adsorption;Electrocatalytic reduction;Grapheme;Niobium phosphate;U(VI)

期刊：

Journal of Hazardous Materials

ISSN：

0304-3894

年：

2023

卷：

442

页码：

130054

DOI：

10.1016/j.jhazmat.2022.130054

基金类别：

CRediT authorship contribution statement Yun Liao: Conceptualization, Methodology, Formal analysis, acquisition, Writing – original draft. Ruilin Lei: Investigation, Methodology, Data curation. Xiaofang Weng: Investigation, Methodology, Data curation. Chuan Yan: Validation, Investigation, Data curation. Jiaxi Fu: Validation, Formal analysis. Guoxing Wei: Formal analysis. Chen Zhang: Visualization. Meng Wang: Conceptualization, Methodology, acquisition, Writing – review & editing. Hongqing Wang: Supervision, Project

机构署名：

本校为第一机构

院系归属：

化学化工学院

核科学技术学院

摘要：

As an energy-efficient and eco-friendly technique, capacitive deionization (CDI) has shown great potential for uranium (U(VI)) capture recently. However, extracting U(VI) with high kinetics, capacity and selectivity remains a major challenge due to the current surface active sites-based material and co-existing ions in aqueous solution. Here we rationally designed a layered 2D/2D niobium phosphate/holey graphene (HGNbP) electrode material, and originally demonstrated its efficient U(VI) capture ability via an electro-adsorption and electrocatalytic reduction coupling process. The less-accumula...

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Uranium capture by a layered 2D/2D niobium phosphate/holey graphene architecture via an electro-adsorption and electrocatalytic reduction coupling process

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