Small-scale measurements of the radon exhalation rate using the flow-through and closed-loop methods were conducted on the surface of a uranium tailing pond to better understand the differences between the two methods. An abnormal radon exhalation behavior was observed, leading to computational fluid dynamics (CFD)-based simulations in which dynamic radon migration in a porous medium and accumulation chamber was considered. Based on the in-situ experimental and numerical simulation results, variations in the radon exhalation rate subject to permeability, flow rate, and insertion depth were qua...