Copper-mediated trifluoromethylation of arylboronic acids by trifluoromethyl sulfonium salts

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成果类型：

期刊论文

作者：

Zhang, Cheng-Pan;Cai, Ji;Zhou, Chang-Bing;Wang, Xiao-Ping;Zheng, Xing;...

通讯作者：

Xiao, Ji-Chang

作者机构：

[Zhou, Chang-Bing; Xiao, Ji-Chang; Wang, Xiao-Ping; Cai, Ji; Zhang, Cheng-Pan] Chinese Acad Sci, Shanghai Inst Organ Chem, Key Lab Organofluorine Chem, Shanghai 200032, Peoples R China.

[Wang, Xiao-Ping; Zheng, Xing] Univ S China, Inst Pharm & Pharmacol, Hengyang, Hunan, Peoples R China.

[Gu, Yu-Cheng] Syngenta, Jealotts Hill Int Res Ctr, Bracknell RG42 6EY, Berks, England.

[Xiao, Ji-Chang] Chinese Acad Sci, Shanghai Inst Organ Chem, Key Lab Organofluorine Chem, 345 Lingling Rd, Shanghai 200032, Peoples R China.

通讯机构：

[Xiao, Ji-Chang] C

Chinese Acad Sci, Shanghai Inst Organ Chem, Key Lab Organofluorine Chem, 345 Lingling Rd, Shanghai 200032, Peoples R China.

语种：

英文

期刊：

Chemical Communications

ISSN：

1359-7345

年：

2011

卷：

期：

页码：

9516-9518

DOI：

10.1039/c1cc13460d

基金类别：

Chinese Academy of SciencesChinese Academy of Sciences; National Natural Science FoundationNational Natural Science Foundation of China (NSFC) [20972179, 21032006]; Syngenta PhD Studentship Award

机构署名：

本校为其他机构

院系归属：

药学与生物科学学院

摘要：

The ligand-free trifluoromethylation of arylboronic acids with a [Ph 2SCF 3] +[OTf] -/Cu(0) system has been carefully investigated. Aryl-, alkenyl- and heteroarylboronic acids with a variety of functional groups were suitable substrates for this reaction. It is suggested that a CuCF 3 species is formed under the reaction conditions....

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Copper-mediated trifluoromethylation of arylboronic acids by trifluoromethyl sulfonium salts

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