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成果类型:
期刊论文
作者:
Liu, Linshuai;Chen, Lifeng;Thummavichai, Kunyapat;Ye, Zhenxiong;Wang, Youbin;...
通讯作者:
Wang, XP
作者机构:
[Ye, Zhenxiong; Fujita, Toyohisa; Wang, Xinpeng; Wang, XP; Wang, Youbin; Liu, Linshuai] Guangxi Univ, Sch Resources Environm & Mat, State Key Lab Featured Met Mat & Life cycle Safety, Nanning 530004, Peoples R China.
[Chen, Lifeng] Univ South China, Sch Nucl Sci & Technol, 28 Changsheng West Rd, Hengyang 421001, Peoples R China.
[Thummavichai, Kunyapat] Northumbria Univ, Fac Engn & Environm, Newcastle Upon Tyne NE1 8ST, England.
通讯机构:
[Wang, XP ] G
Guangxi Univ, Sch Resources Environm & Mat, State Key Lab Featured Met Mat & Life cycle Safety, Nanning 530004, Peoples R China.
语种:
英文
关键词:
MOF-on-MOF;Radioactive iodine;Amine functionalization;Adsorption;DFT
期刊:
Chemical Engineering Journal
ISSN:
1385-8947
年:
2023
卷:
474
页码:
145858
基金类别:
This work was supported by the National Natural Science Foundation of China [grant numbers 21866007, 12075066]. CRediT authorship contribution statement Linshuai Liu: Writing – original draft. Lifeng Chen: Formal analysis, Writing – review & editing. Kunyapat Thummavichai: Formal analysis, Writing – review & editing. Zhenxiong Ye: Investigation. Youbin Wang: Methodology, Conceptualization. Toyohisa Fujita: Supervision. Xinpeng Wang: acquisition.
机构署名:
本校为其他机构
院系归属:
核科学技术学院
摘要:
The effective capture of radioactive iodine vapor is crucial for radiation safety during spent fuel reprocessing. However, current materials used for iodine vapor capture have limitations such as low adsorption efficiency and poor stability, which hinder the effectiveness. To address this issue, an efficient, stable, recoverable and heterogeneous MOF-on-MOF [NH2-MIL-101-on-NH2-UiO-66] adsorbent was prepared using the epitaxial growth strategy. The adsorbent was extensively characterized with various technologies including FT-IR, XPS and XRD, and batch experiments were conducted to evaluate the...

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